| Field |
Field Value |
| Title |
Pharmaceutical and personal care products in groundwater, subsurface drainage, soil, and wheat grain, following a high single application of municipal biosolids to a field |
| Type |
Journal Article |
| Abstract |
Dewatered municipal biosolids (DMBs) were applied to a field at a rate of 22 Mg dw ha-1 in October 2008. Pharmaceuticals and personal care products (PPCPs) were monitored in groundwater, tile drainage, soil, DMB aggregates incorporated into the soil post-land application, and in the grain of wheat grown on the field for a period of 1 year following application. Over 80 PPCPs were analyzed in the source DMB. PPCPs selected for in-depth monitoring included: antibiotics (tetracyclines, fluoroquinolones), bacteriocides
(triclosan, triclocarban), beta-blockers (atenolol, propranolol, metaprolol), antidepressants (fluoxetine, citalopram, venlafaxine, sertraline), antifungals (miconazole), analgesics (acetaminophen, ibuprofen) and anticonvulsants (carbamazepine). PPCPs in tile were observed twice, 3 weeks and 2 months post-application. Of all PPCPs measured in tile drainage, only carbamazepine, ibuprofen, acetaminophen, triclosan, triclocarban, venlafaxine, and citalopram were detected (5-74 ng L-1). PPCPs were not detected in groundwater >2 m depth below the soil surface, and concentrations above detection limits at 2 m depth were only observed once just after the first rain event post-application. In groundwater, all compounds found in tile, except carbamazepine, acetaminophen and citalopram, were detected (10- 19 ng L-1). PPCPs were detected in DMB aggregates incorporated in soil up to 1 year post-application, with miconazole and fluoxetine having the lowest percent reductions over 1 year (50%). For several compounds in these aggregates, concentration declines were of exponential decay form. No PPCPs were detected in the grain of wheat planted post-application on the field. No PPCPs were ever detected in water, soil or grain samples from the reference plot, where no DMB was applied. |
| Document Number |
BIN.PCPP.5.9 |
| Book Title |
|
| Pages |
194-203 |
| Conference Name |
|
| Editor |
|
| Conference Location |
|
| Keywords |
pharmaceutical, personal care products, PPCPs, groundwater, drainage, soil, wheat grain, incorporated, concentrations |
| Date |
2012 |
| Publisher |
|
| Volume |
87 |
| Journal |
Chemosphere |
| Author |
Gottschall, N., E. Topp, C. Metcalfe, M. Edwards, M. Payne, S. Kleywegt, P. Russell, D.R. Lapen |
| Institution |
|
| Type of Work |
|
| Place Published |
|
| Report Number |
|
| University |
|
| Thesis Type |
|
| Magazine |
|
| Newspaper |
|
| Issue |
|
| Label |
|